Anthropogenic radionuclides in atmospheric air over Switzerland during the last few decades.
Details
Serval ID
serval:BIB_A33884CDAE90
Type
Article: article from journal or magazin.
Collection
Publications
Institution
Title
Anthropogenic radionuclides in atmospheric air over Switzerland during the last few decades.
Journal
Nature Communications
ISSN
2041-1723 (Electronic)
ISSN-L
2041-1723
Publication state
Published
Issued date
2014
Volume
5
Pages
3030
Language
english
Notes
Publication types: Journal Article
Abstract
The atmospheric nuclear testing in the 1950s and early 1960s and the burn-up of the SNAP-9A satellite led to large injections of radionuclides into the stratosphere. It is generally accepted that current levels of plutonium and caesium radionuclides in the stratosphere are negligible. Here we show that those radionuclides are present in the stratosphere at higher levels than in the troposphere. The lower content in the troposphere reveals that dry and wet deposition efficiently removes radionuclides within a period of a few weeks to months. Since the stratosphere is thermally stratified and separated from the troposphere by the tropopause, radioactive aerosols remain longer. We estimate a mean residence time for plutonium and caesium radionuclides in the stratosphere of 2.5-5 years. Our results also reveal that strong volcanic eruptions like Eyjafjallajökull in 2010 have an important role in redistributing anthropogenic radionuclides from the stratosphere to the troposphere.
Pubmed
Web of science
Open Access
Yes
Create date
21/03/2014 18:58
Last modification date
20/08/2019 15:08